The Klingons got smoothe heads for TOS from Kingon doctors trying to create “augments” [Augmented Klingons] from human augment DNA - ST Enterprise, season 3 or 4
They got bumpy heads again because they cured the “augments” virus [alluded to at the end of the augment arc in ST Enterprise]
Real reason was TOS had a crappy budget and couldn’t afford the prosthetic foreheads.