The general level of airborne aerosols and soot particles must have been far higher in the late 19th and early 20th century, even accounting for the increase in population, due to dependence on coal and wood for heat to warm buildings and drive steam engines and electric power plants. In my lifetime, I have watched the skies clear. Once, while driving through Steubenville, Ohio I asked someone there why the buildings were so blackened on the walls and rooftops and he simply said, "The steel plant."
Your observations are quite valid.